273:
efficiency. Furthermore, he investigated the hydrogenation of functionalized aromatic compounds using water-dispersed Rh nanoparticles stabilized with PVP and demonstrated the ability to control chemoselectivity in Rh nanoparticle catalysts by selectively poisoning sites with phosphine ligands. Additionally, he presented a technique for the direct hydrogenation of carbon dioxide into formic acid through the utilization of a homogeneous ruthenium catalyst in an aqueous medium containing dimethyl sulphoxide (DMSO), without the inclusion of any supplementary substances. In 2017, he collaborated with
Yuichiro Himeda and others and introduced an approach utilizing formic acid as a hydrogen donor, combined with iridium catalysts and electronically tailored ligands, to enhance the selectivity of methanol synthesis from carbon dioxide (CO
299:
to immobilize the catalyst, ruthenium-TPPTS, including ion exchange, coordination, and physical absorption techniques. His collaborative research with
Matthias Beller and others established formic acid as an ideal hydrogen storage material due to its liquid state at room temperature and non-toxic properties. His assessment of cesium formate and bicarbonate salts for hydrogen storage and transportation demonstrated that combining bicarbonate hydrogenation and formate decomposition reactions in water offered viable and replenishable hydrogen battery solutions. While evaluating the progress in catalytic processes for efficient hydrogen storage and utilization, his work focused on liquid-based systems such as formic acid and alcohol and highlighted significant advancements in CO
312:
changes. Focusing on the stopped-flow technique, he conducted research on the interactions between specific divalent transition metal ions and also developed a high-pressure stopped-flow spectrometer capable of studying rapid reactions using absorbance and fluorescence detection. In related research, his study established the role of the dimeric form of 1-methoxy-3-methyl carbonatotetrabutyldistannoxane as an intermediate in synthesizing dimethyl carbonate, while also highlighting the potential existence of a novel trinuclear di-n-butyltin(IV) compound, possibly derived from the organometallic precursor n-Bu
277:). More recently in 2018, he addressed the problem of reducing energy-intensive processes in the production of lignin-derived chemicals by developing a technique that utilized precisely engineered Rh nanoparticles evenly distributed within sub-micrometer carbon hollow spheres for the targeted reduction of lignin-derived substances at moderate temperatures.
298:
Laurenczy's hydrogen storage research has led to the development of hydrogen storage technologies. He investigated the immobilization of a highly efficient homogeneous catalyst used in the formic acid decomposition process to produce hydrogen and carbon dioxide and outlined different methods employed
289:
pressures. Focusing his research efforts on selective dehydrogenation of HCOOH, he investigated the correlation between the stability and effectiveness of catalysts in the process of formic acid dehydrogenation, and developed a catalytic framework designed to facilitate the precise dehydrogenation of
216:
at the
Université de Bourgogne in 2007. In 2010, he was appointed as Professor at the École Polytechnique Fédérale de Lausanne, a role that he served until 2019. As of 2019, he is the professor emeritus at the École Polytechnique Fédérale de Lausanne. In 2022, he was elected as an External Member of
336:
Laurenczy's research on reaction mechanisms has resulted in an improved understanding of catalytic reactions and synthetic methodologies, including the design of efficient and selective transformations, as well as the synthesis of complex molecules with applications in medicine, materials science.
311:
During his investigation of the Bray reaction in enclosed environments and the influence of elevated pressure on the reaction, Laurenczy discovered that oxygen acts as an independent species and demonstrated that subjecting the reaction to high pressure (2000 bar) induced significant oscillation
272:
hydrogenation utilizing a ruthenium dihydride complex, while identifying crucial intermediates, emphasizing the significance of the trans-form of the complex, and highlighting the importance of preserving formate ion stability and ensuring efficient formic acid removal to enhance catalytic
263:
Lauranczy's research on the
Hydrogenation of compounds has focused on developing new catalysts, elucidating reaction mechanisms, optimizing processes, overcoming challenges in hydrogenating specific substrates, and enabling selective transformations. He evaluated the effectiveness of
280:
Laurenczy's dehydrogenation research has concentrated on the quantitative dehydrogenation of formic acid in an aqueous solution using iron as catalysts. Moreover, he examined the process of formic acid dehydrogenation facilitated by water-soluble complexes of ruthenium
324:. In his investigation of the catalytic capability of a uniform iridium compound in the formic acid disproportionation process, leading to methanol production, he demonstrated the potential for high yields and achieved yields of up to 75% in deuterium oxide (D
337:
Moreover, his examination of aqueous catalytic reactions demonstrated successful transmission of carbon dioxide into formic acid and methanol utilizing an iridium complex within an aqueous medium, while operating under ambient temperatures.
364:
Scolaro, C., Bergamo, A., Brescacin, L., Delfino, R., Cocchietto, M., Laurenczy, G., ... & Dyson, P. J. (2005). In vitro and in vivo evaluation of ruthenium (II)− arene PTA complexes. Journal of medicinal chemistry, 48(12),
374:
Sordakis, K., Tang, C., Vogt, L. K., Junge, H., Dyson, P. J., Beller, M., & Laurenczy, G. (2018). Homogeneous catalysis for sustainable hydrogen storage in formic acid and alcohols. Chemical
Reviews, 118(2),
360:
Boddien, A., Mellmann, D., Gärtner, F., Jackstell, R., Junge, H., Dyson, P. J., Laurenczy, G., ... & Beller, M. (2011). Efficient dehydrogenation of formic acid using an iron catalyst. Science, 333(6050),
356:
Fellay, C., Dyson, P. J., & Laurenczy, G. (2008). A viable hydrogen‐storage system based on selective formic acid decomposition with a ruthenium catalyst. Angewandte Chemie
International Edition, 47(21),
668:"Formation and Characterization of Water-Soluble Hydrido-Ruthenium(II) Complexes of 1,3,5-Triaza-7-phosphaadamantane and Their Catalytic Activity in Hydrogenation of CO 2 and HCO 3 - in Aqueous Solution"
1781:"Aqueous catalytic dimerisation of ethylene: characterization of the reaction intermediates [Ru(CH2CH2)(H2O)5](tos)2 and [Ru(CH2CH2)2(H2O)4](tos)2(tos = toluene-p-sulfonate)"
1029:"Direct, in situ determination of pH and solute concentrations in formic acid dehydrogenation and CO2 hydrogenation in pressurised aqueous solutions using 1H and 13C NMR spectroscopy"
208:. In 1985 he moved to Switzerland (UNIL). In 1991, he made his habilitation (Hungarian Academy of Sciences, Budapest). In the same year, he was appointed as Maître Assistant at the
1740:
Scolaro, Claudine; Bergamo, Alberta; Brescacin, Laura; Delfino, Riccarda; Cocchietto, Moreno; Laurenczy, Gábor; Geldbach, Tilmann J.; Sava, Gianni; Dyson, Paul J. (June 16, 2005).
371:
Moret, Séverine, Dyson, Paul J., Laurenczy, Gábor, (2014). Direct synthesis of formic acid from carbon dioxide by hydrogenation in acidic media. Nature
Communications. 5 (1): 4017.
941:
Boddien, Albert; Mellmann, Dörthe; Gärtner, Felix; Jackstell, Ralf; Junge, Henrik; Dyson, Paul J.; Laurenczy, Gábor; Ludwig, Ralf; Beller, Matthias (September 23, 2011).
480:
Federsel, Christopher; Boddien, Albert; Jackstell, Ralf; Jennerjahn, Reiko; Dyson, Paul J.; Scopelliti, Rosario; Laurenczy, Gabor; Beller, Matthias (December 10, 2010).
158:
120:
1579:"Monocomplex formation and dissociation of some first row divalent transition metal ions with 2-chloro-1,10-phenanthroline by the high-pressure stopped-flow technique"
1144:
Guerriero, Antonella; Bricout, Hervé; Sordakis, Katerina; Peruzzini, Maurizio; Monflier, Eric; Hapiot, Frédéric; Laurenczy, Gábor; Gonsalvi, Luca (September 5, 2014).
368:
Grasemann, M., & Laurenczy, G. (2012). Formic acid as a hydrogen source–recent developments and future trends. Energy & Environmental
Science, 5(8), 8171–8181.
1398:
Boddien, Albert; Federsel, Christopher; Sponholz, Peter; Mellmann, Dörthe; Jackstell, Ralf; Junge, Henrik; Laurenczy, Gabor; Beller, Matthias (September 20, 2012).
1604:
Bugnon, P.; Laurenczy, G.; Ducommun, Y.; Sauvageat, P. Y.; Merbach, A. E.; Ith, R.; Tschanz, R.; Doludda, M.; Bergbauer, R.; Grell, E. (September 1, 1996).
1276:"Hydrogen storage and delivery: Immobilization of a highly active homogeneous catalyst for the decomposition of formic acid to hydrogen and carbon dioxide"
268:) and bicarbonate ions in an aqueous solution by employing a water-soluble ruthenium(II) complex. In a collaborative study, he explored the pathways of CO
1645:"Di-n-butyltin(IV)-catalyzed dimethyl carbonate synthesis from carbon dioxide and methanol: An in situ high pressure 119Sn{1H} NMR spectroscopic study"
264:
hydrido-ruthenium(II) complexes as catalysts in hydrogenation reactions and investigated the catalytic hydrogenation process of carbon dioxide (CO
1367:"A Viable Hydrogen Storage and Release System Based on Cesium Formate and Bicarbonate Salts: Mechanistic Insights into the Hydrogen Release Step"
1431:"Chemical Equilibria in Formic Acid/Amine-CO2 Cycles under Isochoric Conditions using a Ruthenium(II) 1,2-Bis(diphenylphosphino)ethane Catalyst"
578:
1468:
Sordakis, Katerina; Tang, Conghui; Vogt, Lydia K.; Junge, Henrik; Dyson, Paul J.; Beller, Matthias; Laurenczy, Gábor (January 24, 2018).
1293:
Boddien, Albert; Gartner, Felix; Mellmann, Dorthe; Sponholz, Peter; Junge, Henrik; Laurenczy, Gábor; Beller, Matthias (June 22, 2011).
303:
hydrogenation and dehydrogenation reactions, with a strong emphasis on the development of sustainable and Earth-abundant catalysts.
1837:
Sordakis, Katerina; Tsurusaki, Akihiro; Iguchi, Masayuki; Kawanami, Hajime; Himeda, Yuichiro; Laurenczy, Gábor (October 24, 2016).
871:
Tsurusaki, Akihiro; Murata, Kazuhisa; Onishi, Naoya; Sordakis, Katerina; Laurenczy, Gábor; Himeda, Yuichiro (February 3, 2017).
430:
482:"A well-defined iron catalyst for the reduction of bicarbonates and carbon dioxide to formates, alkyl formates, and formamides"
281:
m-triphenylphosphinetrisulfonate (TPPTS) and contributed to the understanding of the carbon dioxide-formic acid systems under H
212:, followed by an appointment as a maître d'enseignement et de recherche at the same institution in 1997. He also served as the
1146:"Hydrogen Production by Selective Dehydrogenation of HCOOH Catalyzed by Ru-Biaryl Sulfonated Phosphines in Aqueous Solution"
35:
229:
storage & generation, catalytic activation of small molecules, the development of medium and high-pressure equipment,
1606:"High-pressure stopped-flow spectrometer for kinetic studies of fast reactions by absorbance and fluorescence detection"
1887:
777:"Carbon Dioxide Hydrogenation Catalyzed by a Ruthenium Dihydride: A DFT and High-Pressure Spectroscopic Investigation"
255:. In addition, he has authored numerous publications, including book chapters and articles in peer-reviewed journals.
707:"In situ NMR characterisation of an intermediate in the catalytic hydrogenation of CO2 and HCO3- in aqueous solution"
1066:
Thevenon, Arnaud; Frost-Pennington, Ewan; Weijia, Gan; Dalebrook, Andrew F.; Laurenczy, Gábor (November 22, 2014).
736:
Federsel, Christopher; Jackstell, Ralf; Boddien, Albert; Laurenczy, Gabor; Beller, Matthias (September 24, 2010).
1068:"Formic Acid Dehydrogenation Catalysed by Tris(TPPTS) Ruthenium Species: Mechanism of the Initial "Fast" Cycle"
1175:
Dalebrook, Andrew F.; Gan, Weijia; Grasemann, Martin; Moret, Séverine; Laurenczy, Gábor (September 5, 2013).
1892:
1707:"Carbon monoxide solubility in ionic liquids: determination, prediction and relevance to hydroformylation"
209:
873:"Investigation of Hydrogenation of Formic Acid to Methanol using H 2 or Formic Acid as a Hydrogen Source"
524:"A viable hydrogen-storage system based on selective formic acid decomposition with a ruthenium catalyst"
453:
233:
catalysts, and reactions with water-soluble compounds. He holds patents to numerous projects including
1807:
1780:
1644:
1578:
1509:"Recent progress for reversible homogeneous catalytic hydrogen storage in formic acid and in methanol"
1508:
1257:"Heterogeneous Silica-Supported Ruthenium Phosphine Catalysts for Selective Formic Acid Decomposition"
997:
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597:
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954:
827:
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1335:
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1107:"CO2 as a hydrogen vector – transition metal diamine catalysts for selective HCOOH dehydrogenation"
235:
205:
193:
95:
83:
1706:
902:
Chen, Lu; Muyden, Antoine P. van; Cui, Xinjiang; Laurenczy, Gabor; Dyson, Paul J. (May 26, 2020).
1674:
Sordakis, K.; Tsurusaki, A.; Iguchi, M.; Kawanami, H.; Himeda, Y.; Laurenczy, G. (May 22, 2017).
1528:
1450:
1087:
978:
923:
648:
445:
1216:"Selective formic acid decomposition for high-pressure hydrogen generation: a mechanistic study"
185:
188:
in
Chemistry from Kossuth University (Debrecen, Hungary) in 1978. Subsequently, he pursued his
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1808:"A new variable temperature and pressure infrared cell to study liquid and liquid–gas systems"
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176:. He is the recipient of the Rudolf Fabinyi Memorial Prize by The Hungarian Chemical Society.
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213:
466:
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Onishi, Naoya; Laurenczy, Gábor; Beller, Matthias; Himeda, Yuichiro (October 15, 2018).
958:
831:
1469:
998:"Quantitative aqueous phase formic acid dehydrogenation using iron(II) based catalysts"
848:
815:
243:
1823:
1590:
942:
816:"Direct synthesis of formic acid from carbon dioxide by hydrogenation in acidic media"
613:
596:
Laurenczy, Gábor; Helm, Lothar; Merbach, André E.; Ludi, Andreas (November 15, 1991).
1876:
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1532:
1256:
996:
Montandon-Clerc, Mickael; Dalebrook, Andrew F.; Laurenczy, Gábor (November 1, 2016).
927:
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246:
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1470:"Homogeneous Catalysis for Sustainable Hydrogen Storage in Formic Acid and Alcohols"
1454:
1275:
1091:
982:
872:
1547:
1430:
705:
Laurenczy, Gábor; Jedner, Stephanie; Alessio, Enzo; Dyson, Paul J. (May 1, 2007).
562:
393:
722:
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775:
Urakawa, Atsushi; Jutz, Fabian; Laurenczy, Gábor; Baiker, Alfons (May 7, 2007).
250:
140:
50:
1013:
1524:
1429:
Sordakis, Katerina; Beller, Matthias; Laurenczy, Gábor, eds. (June 22, 2014).
102:
1365:
Sordakis, Katerina; Dalebrook, Andrew F.; Laurenczy, Gábor (August 3, 2015).
1214:
Fellay, Céline; Yan, Ning; Dyson, Paul J.; Laurenczy, Gábor (June 22, 2009).
1145:
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629:"A Precious Catalyst: Rhodium‐Catalyzed Formic Acid Dehydrogenation in Water"
1741:
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1839:"Carbon Dioxide to Methanol: The Aqueous Catalytic Way at Room Temperature"
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904:"Selective hydrogenation of lignin-derived compounds under mild conditions"
857:
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761:
753:
691:
644:
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161:. He is academician, External Member of the Hungarian Academy of Sciences.
1336:"Formic acid as a hydrogen source – recent developments and future trends"
1792:
412:
226:
154:
147:
64:
1676:"Aqueous phase homogeneous formic acid disproportionation into methanol"
1563:
204:
Laurenczy began his academic career in 1984 in
Kossuth University as an
1806:
Laurenczy, Gábor; Lukács, Ferenc; Roulet, Raymond (February 27, 1998).
1691:
1415:
1351:
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839:
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136:
60:
46:
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1742:"In vitro and in vivo evaluation of ruthenium(II)-arene PTA complexes"
1643:
Laurenczy, Gábor; Picquet, Michel; Plasseraud, Laurent (May 1, 2011).
1621:
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Laurenczy, Gábor; Bugnon, Pascal; Merbach, André E. (August 1, 1992).
1161:
683:
1718:
561:
Laurenczy, Gabor; Fellay, Celine; Dyson, Paul, eds. (June 22, 2008).
1705:
Ohlin, C. André; Dyson, Paul J.; Laurenczy, Gábor (April 28, 2004).
346:
2022 – Rudolf Fabinyi Memorial Prize, The Hungarian Chemical Society
1027:
Moret, Séverine; Dyson, Paul J.; Laurenczy, Gábor (March 6, 2013).
666:
Laurenczy, Gábor; Joó, Ferenc; Nádasdi, Levente (October 1, 2000).
814:
Moret, Séverine; Dyson, Paul J.; Laurenczy, Gábor (June 2, 2014).
522:
Fellay, Céline; Dyson, Paul J.; Laurenczy, Gábor (June 22, 2008).
189:
91:
943:"Efficient Dehydrogenation of Formic Acid Using an Iron Catalyst"
598:"The binding of dinitrogen to ruthenium(II) in aqueous solution"
230:
738:"Ruthenium-catalyzed hydrogenation of bicarbonate in water"
1785:
Journal of the Chemical Society, Chemical Communications
1274:
Gan, Weijia; Dyson, J. Paul; Laurenczy, Gábor (2008).
1255:
Gan, Weijia; Dyson, J. Paul; Laurenczy, Gábor (2013).
1334:
Grasemann, Martin; Laurenczy, Gábor (July 18, 2012).
1105:Fink, Cornel; Laurenczy, Gábor (January 31, 2017).
164:Laurenczy's research interests lie in the field of
116:
111:
101:
79:
74:
56:
42:
28:
21:
1546:Laurenczy, Gabor; Beck, Mihaly T. (May 22, 1994).
1779:Laurenczy, G.; Merbach, A. E. (January 1, 1993).
196:at the same institution, completing it in 1980.
1400:"Towards the development of a hydrogen battery"
1295:"Hydrogen storage in formic acid amine adducts"
1177:"Hydrogen storage: beyond conventional methods"
627:Fink, Cornel; Laurenczy, Gábor (May 15, 2019).
1548:"Effect of High Pressure on the Bray Reaction"
259:Hydrogenation and dehydrogenation of compounds
8:
290:formic acid within an aqueous environment.
168:, primarily focusing on hydrogen storage,
18:
16:Hungarian chemist and academic (born 1954)
1382:
1310:
1231:
847:
225:Laurenczy is most known for his works on
159:École Polytechnique Fédérale de Lausanne
121:École Polytechnique Fédérale de Lausanne
1280:Reaction Kinetics and Catalysis Letters
633:European Journal of Inorganic Chemistry
528:Angewandte Chemie International Edition
486:Angewandte Chemie International Edition
385:
462:
451:
431:"Fabinyi Rudolf Emlékérem díjazottjai"
407:
405:
403:
517:
515:
7:
564:Hydrogen production from formic acid
1649:Journal of Organometallic Chemistry
446:"Double honors for Gabor Laurenczy"
217:the Hungarian Academy of Sciences.
1404:Energy & Environmental Science
1340:Energy & Environmental Science
711:Inorganic Chemistry Communications
172:and catalytic activation of small
14:
1552:The Journal of Physical Chemistry
444:Papageorgiou, Nik (May 5, 2022).
1661:10.1016/j.jorganchem.2011.02.010
413:"EPFL People – Gabor Laurenczy"
394:"Az MTA köztestületének tagjai"
1843:Chemistry - A European Journal
1746:Journal of Medicinal Chemistry
1513:Coordination Chemistry Reviews
781:Chemistry - A European Journal
1:
1824:10.1016/S0003-2670(97)00696-X
1591:10.1016/S0020-1693(00)92357-0
1220:Chemistry: A European Journal
614:10.1016/S0020-1693(00)80178-4
307:High pressure kinetic studies
723:10.1016/j.inoche.2007.01.020
1486:10.1021/acs.chemrev.7b00182
36:Hungarian People's Republic
1909:
1014:10.1016/j.jcat.2015.11.012
1525:10.1016/j.ccr.2017.11.021
328:O) through this process.
126:
70:
889:10.1021/acscatal.6b03194
1711:Chemical Communications
1583:Inorganica Chimica Acta
1312:10.2533/chimia.2011.214
1181:Chemical Communications
967:10.1126/science.1206613
602:Inorganica Chimica Acta
1855:10.1002/chem.201603407
1812:Analytica Chimica Acta
1447:10.1002/cctc.201300740
1384:10.1002/cctc.201500625
1233:10.1002/chem.200801824
1084:10.1002/cctc.201402410
793:10.1002/chem.200601339
754:10.1002/cssc.201000151
645:10.1002/ejic.201900344
540:10.1002/anie.200800320
498:10.1002/anie.201004263
461:Cite journal requires
210:University of Lausanne
1263:. pp. 3124–3130.
820:Nature Communications
1793:10.1039/C39930000187
1610:Analytical Chemistry
1585:. 198–200: 159–164.
1002:Journal of Catalysis
1849:(44): 15605–15608.
1564:10.1021/j100071a004
1282:. pp. 205–213.
1111:Dalton Transactions
1033:Dalton Transactions
959:2011Sci...333.1733B
953:(6050): 1733–1736.
832:2014NatCo...5.4017M
672:Inorganic Chemistry
332:Reaction mechanisms
236:Hydrogen production
206:Assistant Professor
194:Inorganic Chemistry
184:Laurenczy earned a
96:Inorganic Chemistry
75:Academic background
1888:Hungarian chemists
1692:10.1039/C6GC03359H
1416:10.1039/C2EE22043A
1352:10.1039/C2EE21928J
1193:10.1039/C3CC43836H
1123:10.1039/C6DT04638J
1045:10.1039/C3DT00081H
920:10.1039/D0GC00121J
840:10.1038/ncomms5017
583:scholar.google.com
214:Visiting Professor
107:Kossuth University
1758:10.1021/jm050015d
1752:(12): 4161–4171.
1686:(10): 2371–2378.
1622:10.1021/ac960382k
1616:(17): 3045–3049.
1558:(20): 5188–5189.
1410:(10): 8907–8911.
1226:(15): 3752–3760.
1187:(78): 8735–8751.
1162:10.1021/cs500655x
1078:(11): 3146–3152.
1039:(13): 4353–4356.
914:(10): 3069–3073.
787:(14): 3886–3899.
684:10.1021/ic000200b
678:(22): 5083–5088.
639:(18): 2381–2387.
579:"Gabor Laurenczy"
534:(21): 3966–3968.
492:(50): 9777–9780.
351:Selected articles
341:Awards and honors
166:reaction kinetics
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1719:10.1039/B401537A
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1474:Chemical Reviews
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1346:(8): 8171–8181.
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294:Hydrogen storage
238:from formic acid
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1680:Green Chemistry
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380:References
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